EAAI Journal 2026 Journal Article
A new mineral quantification method via experiment-enhanced transfer learning of linear mixed mid-infrared spectra data
- Tao Han
- Tengfei Yu
- Peng Lin
- Wen Ma
- Zhenhao Xu
Accurate quantitative mineral analysis is fundamental for understanding geological evolution, predicting rock mechanical behavior, and delineating exploration targets. Mid-infrared spectroscopy offers rapid, non-destructive acquisition of mineralogical information. However, the application of mid-infrared spectroscopy in mineral quantification is still hindered by strong spectral nonlinearity caused by intimate mineral mixtures and the challenges of spectral testing in complex geological conditions. To address these limitations, we proposed a new mineral quantification method via experiment-enhanced transfer learning of linear mixed mid-infrared spectra data (MQM-ExpTL). The proposed method integrates submodel internal transfer and comprehensive fine-tuning strategies to construct a deep learning model capable of robustly quantifying protolith and clay minerals while capturing and interpreting non-linear mixing effects. On the independent test set, our method significantly outperformed support vector regression (SVR), partial least squares regression (PLSR), competitive adaptive reweighted sampling-support vector regression (CARS-SVR), competitive adaptive reweighted sampling-partial least squares regression (CARS-PLSR), the standard transfer learning model, and the model without transfer learning across coefficient of determination (R2), mean squared error (MSE), and mean absolute error (MAE). Specifically, our method achieves an overall prediction accuracy of R2 = 0. 98, yielding an improvement of 0. 9% to 32% over the comparative methods. Furthermore, we elucidated the rationale for adopting the validation loss for hyperparameter optimization and examined the differences in model selection when employing various globally optimal model selection criteria. The method provides an efficient quantitative approach to support the application of mid-infrared spectroscopy in remote sensing interpretation, geological identification, and mineral exploration.